Platinum(Ii) Metallothioneins
Platinum(Ii) Metallothioneins
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The approximate differences in the orientations of these terminal ligands in going from the 3-Zn to the 3-Pt cluster are 90° about the S 4 rotation-reflection axes bisecting the plane of each Zn 2+ and its two terminal ligands. Despite the different orientations of the terminal sulfurs, this 3-Pt cluster can be inserted into the B region of the crystallographic MT structure, without significantly changing the conformation of the polypeptide backbone, by rotations about C a -C R bonds of the nin...e cysteines in this region.
A better fit may be obtained by permitting changes in the Pt-S-Pt bond angles from the idealized 110°.
According to a recent review by Dance [176], bonds angles 110 for M-S-M bonds in metal-thiolate complexes generally vary between about 90-120°. Refinement of the crystal lographic structure in Figure 1-2 from 230 to 190 pm resolution has revealed that the M-S-M bond angles in native MT actually vary from 80-130° [9]. In addition, the net forces of hydrogen-bonding and other weak interactions in the polypeptide backbone of MT probably cause slight distortions from D 4h about the Pt(II) centers.
What to read after Platinum(Ii) Metallothioneins?
You can find similar books in the "Read Also" column, or choose other free books by Bongers, Jacob, 1959- to read onlineMoreLess
To quickly assess the difficulty of the text, read a short excerpt:
The approximate differences in the orientations of these terminal ligands in going from the 3-Zn to the 3-Pt cluster are 90° about the S 4 rotation-reflection axes bisecting the plane of each Zn 2+ and its two terminal ligands. Despite the different orientations of the terminal sulfurs, this 3-Pt cluster can be inserted into the B region of the crystallographic MT structure, without significantly changing the conformation of the polypeptide backbone, by rotations about C a -C R bonds of the nin...e cysteines in this region.
A better fit may be obtained by permitting changes in the Pt-S-Pt bond angles from the idealized 110°.
According to a recent review by Dance [176], bonds angles 110 for M-S-M bonds in metal-thiolate complexes generally vary between about 90-120°. Refinement of the crystal lographic structure in Figure 1-2 from 230 to 190 pm resolution has revealed that the M-S-M bond angles in native MT actually vary from 80-130° [9]. In addition, the net forces of hydrogen-bonding and other weak interactions in the polypeptide backbone of MT probably cause slight distortions from D 4h about the Pt(II) centers.
What to read after Platinum(Ii) Metallothioneins?
You can find similar books in the "Read Also" column, or choose other free books by Bongers, Jacob, 1959- to read onlineMoreLess
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